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Willard Libby (1908–1980), a professor of chemistry at the University of Chicago, began the research that led him to radiocarbon dating in 1945.
He was inspired by physicist Serge Korff (1906–1989) of New York University, who in 1939 discovered that neutrons were produced during the bombardment of the atmosphere by cosmic rays.
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Korff predicted that the reaction between these neutrons and nitrogen-14, which predominates in the atmosphere, would produce carbon-14, also called radiocarbon.